Yes but in your first post you stated you wanted to ground both center taps (X2-X3 and 4-9 on the HV side) on the same transformer which is why I am trying to point out that the grounding of the X2-X3 on the step up transformer or the 4-9 center tap on the step down transformer is totally unnecessary, by only grounding the secondaries (4-9 on the step up, and X2-X3 on the step down) will provide all the fault current path you can ever get, a fault on the 480v lines to ground will only go back to the secondaries of the step up transformer, it will not flow on a EGC connected to the X2-X3 back to the panel, this is because a transformer is isolating and the primary and secondary are isolated from each other, a fault on the 480v lines does not want to return back to the service grounding system, it is only returning to the center tap (4-9) on the secondaries, the same goes for the step down transformer, you only ground the X2-X3 center tap on the secondaries, again for the same reason above there is no reason to ever ground the primary (4-9) on the step down transformer.
Another point is if this was a common core three phase WYE and you grounding the X0 of the primary of the transformer back to the supply grounding and it is also a WYE supply you would have all kinds of circulating currents that would cause overheating of the EGC and the transformer, the NEC does not require the primary of a transformer to be grounded, the reason is the conductors feeding a primary already have a referance to the supply conductors at the suply end, the same goes for the 480v conductors between the two transformers, if you connect the EGC run with these conductors to the center tap on the secondary, you now have just given this EGC a referance to the 480v conductors and a fault will cause current to flow, at the step down transformer you will do this again by connecting an EGC to the X2-X3 on this transformer, not the 120/240 secondaries have a referance to these conductors and this gives them a fault path.
Think of it this way, a ground fault is only a fault between the center tap and one of the phase conductors (hot's), if you were to short one of the hots to the center tap on a secondary of a transformer don't you think you would have a fault?, now attach a EGC to this center tap and short a hot to this EGC do you think current would not flow and open a breaker? yes it will without any EGC to the primary.
Here is how all transformers are run, the EGC run to the step up transformer is sized for the 60 amps supplying the first transformer, it is connected to the transformer case and a jumper is made to the center tap on the secondaries (4-9 Tap) then a EGC is run from this tap with the 480v secondaries sized for the 30 amps, to the step down transformer, it is connected to this transformers case and a jumper is made to the secondary center tap (X2-X3) then an EGC is run from this tap with the secondaries to the load whether it is a breaker panel or just a load, in no case is there any reason to ever connect any EGC to the primary of either transformer.
As was stated there are other requirements in the NEC for grounding electrodes at each SDS (transformer) as well as other requirements, maybe someone could find a graphic that shows the above.
I think this is what Jraef was questioning in post 2 also.