Seems since they’re no neutral to this unit that 240volt delta 3/0 would be best.
I am surprised by how many electricians become somewhat confused when they have to work on systems that do not have 'solid' Line-Neutral and Line-Ground connections tions, so I like to include neutrals.Even though the unit does not need a neutral, it may have a drive. I would go with a 120.240 secondary so you will have the neutral reference.
(or the two previous posts that popped up as I as typing)