The wiring diagram already shows the choice of where to bond the GEC, i.e. which circuit conductor is grounded. Who made that choice? Is this a field installed pair of transformers, or internal to a manufactured and listed piece of equipment?
The more typical choice would be to ground the conductor that is the center-tapped, which you call L1'.
Note also you have labeled a conductor L2/N, but it should not be labeled N. The grounded conductor is not always a neutral, on a 3-phase 3-wire corner grounded delta you have a grounded conductor which is not neutral. The center-tapped conductor, that you call L1', is in fact neutral to L2 and L3.
Cheers, Wayne